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国家自然科学基金(50908097)

作品数:5 被引量:8H指数:2
相关作者:周丹丹王艳龙高琳琳董双石张建宾更多>>
相关机构:吉林大学更多>>
发文基金:国家自然科学基金国家教育部博士点基金中国博士后科学基金更多>>
相关领域:环境科学与工程化学工程理学一般工业技术更多>>

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Suspended solid abatement in a conical fluidized bed flocculator被引量:1
2013年
With the random movement of silica gel beads in a conical fluidized bed, micro-vortices resulting from the fluidization promoted the collision and aggregation of suspended fine kaolin powders. The abatement efficiencies of the suspended fine solids under several hydrodynamic conditions were studied, and a suitable control strategy for operating the conical fluidized bed flocculators was identified. The suspended solids abatement efficiency was found to increase with increasing Camp Number and flocculation time (T), but decreased with the increase of velocity gradient (G) within the range studied in this research (165.1-189.6s-1). The abatement efficiencies were all more than 60% at the range of G = 165-180 s 1 and T = 15-33 s at an initial kaolin solid concentration of 150mg·L-1, polymer aluminum chloride dosage of 60 mg· L -1 and sedimentation time of 20 min. However, the formation of flocs was influenced by the liquid back- mixing. Excessive backmixing caused the breakup of ftocs and resulted in difficulty for the fine powders to aggregate and sediment to the reactor bottom. The results of the calculated fractal dimension and measured free sedimenta- tion velocity of flocs obtained at different runs showed similar flocs properties, and indicated an easy control strategy for sedimentation of the flocs.
Dandan ZHOUShuangshi DONGKeyu LIHuizhong JIANGDandan SHANG
关键词:BEDFLOCCULATIONVELOCITYGRADIENT
球形活性炭负载和Er^(3+):YAlO_3掺杂TiO_2的制备及其在可见光下降解甲基橙(英文)被引量:4
2012年
为使TiO2能够在可见光下发挥其于紫外激发下的高光催化活性,且易于从处理废水中分离,采用溶胶-凝胶法将TiO2与掺杂稀土离子Er3+的上转换发光剂Er3+:YAlO3结合,再将其负载到球形活性炭(SAC)表面,制备出可见光响应的负载型Er3+:YAlO3/TiO2-SAC光催化剂。通过XRD、EDS、SEM与FSA等手段对制备的光催化剂进行晶相、表面结构与元素分布、发光光谱等表征。以甲基橙为目标污染物,研究制备的光催化剂在可见光下的催化活性。结果表明,Er3+:YAlO3可以作为上转换发光材料,它吸收可见光并发射紫外光进而激发TiO2。700°C煅烧制备的催化剂具有最佳的光催化活性,可见光下表观反应速率常数可达0.0197min-1。
董双石张建宾高琳琳王艳龙周丹丹
关键词:可见光上转换发光材料TIO2
基于流态化作用的吸附反应动力学和穿透特征被引量:1
2014年
基于流态化作用的吸附反应动力学和穿透特征研究还鲜见报道.以苯酚为吸附质、活性炭为吸附剂,探讨了不同流态化紊流强度对基于流态化作用的吸附效率、吸附动力学特性、吸附反应穿透曲线和饱和吸附量的影响,并与相同条件的固定床吸附反应器进行了对比研究.结果表明,表观流速为8 mm·s-1和13 mm·s-1时,基于流态化和固定态的活性炭在5 min内的吸附效率均达到93%以上,吸附反应均符合经典二级动力学方程,且其相关系数大于0.999.穿透实验结果表明,表观流速为6 mm·s-1和8 mm·s-1时,基于流态化的活性炭对苯酚的吸附总量分别较固定态高8.77 mg·g-1和24.70 mg·g-1.可见,基于流态化吸附反应器与基于固定态吸附反应器相比,具有吸附反应效率高,吸附总量大的特征.
王君王瑶黄星袁益龙陈瑞晖周航周丹丹
关键词:流态化吸附动力学
Optimization of multi-stage velocity gradients in a cylindrical fluidized bed flocculator
2015年
Flocculation time is conventionally believed to be proportional to the flocculation efficiency of a cylindrical fluidized bed flocculator.However,in a single-stage velocity gradient situation,the flocculation efficiency decreases when the optimal flocculation time is exceeded.A multi-stage velocity gradient was established in a cylindrical fluidized bed flocculator,based on the hydraulic classification theory.This multi-stage velocity gradient fluidized bed flocculator(MGF) created a more suitable environment for floc growth and protection,which was confirmed by the size distribution of flocs along the bed height.Correspondingly,the abatement efficiencies for Kaolin slurry and dyed wastewater treatment in the MGF were enhanced by5-10%,and by 7-20%,respectively,compared with those in the single-stage velocity gradient fluidized bed flocculators(SGFs).The initial bed height distribution ratio along the velocity gradients was an important factor for MGF optimization.
Yamei LuJun WangDandan ZhouZhengxue XuXiaotao T.Bi
关键词:流化床染色废水处理
Anti-shock loading capability of a fluidized-bed flocculator被引量:2
2012年
The efficiency of a fluidized-bed flocculator with 800- m particles of 1360 kg/m3 in density was studied, and the anti-shock capability of the unit was estimated for three kinds of industrial wastewater: heavy turbidity wastewater, dispersed dyeing wastewater and starch wastewater. Steady removal efficiency was contributed by the following characteristics of the flocculator: (1) the dynamic conditions, flocculation time and velocity gradient, which were stabilized at a steady level as the loading rate changed; (2) hydrodynamic characteristics, especially the considerable rise of expanded bed height with increasing superficial velocity when small and light particles were employed as the solid phase; (3) flocs growth characteristics in the fluidized bed, which caused the density and size of the flocs being maintained at a compensational relationship, resulted the stabilized settling velocity of the flocs.
Dandan ZhouShuangshi DongYang YangWenyuan ZhaoLinlin Gao
关键词:休克工业废水
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