In this paper, ultracold atoms and molecules in a dark magneto-optical trap （MOT） are studied via depumping the cesium cold atoms into the dark hyperfine ground state. The collision rate is reduced to 0.45 s-1 and the density of the atoms is increased to 5.6 × 1011 cm-3 when the fractional population of the atoms in the bright hyperfine ground state is as low as 0.15. The vibrational spectra of the ultracold cesium molecules are also studied in a standard MOT and in a dark MOT separately. The experimental results are analyzed by using the perturbative quantum approach.
The Stark structures in a cesium atom around n=18 are numerically calculated. The results show that the components of 20D states with a small azimuthal quantum number ｜m｜ shift upward a lot, and those with a large ｜m｜ shift downward a little within 1100 V/cm. All components of P states shift downward. Experimental work has been performed in ultracold atomic cesium. Atoms initially in 6P3/2 state are excited to high-n Rydberg states by a polarization light perpendicular to the field, and Stark spectra with ｜m｜=1/2,3/2,5/2 are simultaneously observed with a large linewidth for the first time. The observed spectra are analyzed in detail. The relative transition probability is calculated. The experimental results are in good agreement with our numerical computation.
